Studie evoluce laserem indukovaného plazmatu pomocí komplementárních a spektroskopických metod

but.committeeprof. RNDr. Radim Chmelík, Ph.D. (předseda) prof. Ing. Miroslav Pouzar, Ph.D. (člen) doc. Mgr. Karel Novotný, Ph.D. (člen) Mgr. Michaela Kuchynka, Ph.D. (člen) doc. Ing. Miroslav Kolíbal, Ph.D. (člen)cs
but.defenceMotivací práce bylo rozšíření LIBS analýzy komplementárními metodami ideálně umožňujícím získat data z jediné ablace (direct plasma imaging, shadowgraphy, sound analysis). Cílů bylo dosařeno a výsledky byly publikovány ve významných mezinárodních časopisech prostřednictvím tří prvoaatorských článků kandidáta. Výsledky jsou významné pro věděcký i aplikací provoz v oblasti LIBS analýzy.cs
but.jazykangličtina (English)
but.programFyzikální a materiálové inženýrstvícs
but.resultpráce byla úspěšně obhájenacs
dc.contributor.advisorKaiser, Jozefen
dc.contributor.authorBuday, Jakuben
dc.contributor.refereeNovotný, Karelen
dc.contributor.refereePouzar, Miroslaven
dc.date.accessioned2024-07-04T03:58:31Z
dc.date.available2024-07-04T03:58:31Z
dc.date.createdcs
dc.description.abstractLaser-Induced Breakdown Spectroscopy (LIBS) is a method of analytical chemistry that provides a qualitative and quantitative sample analysis. As this method has been implemented in more and more applications, certain limitations and drawbacks have been raised from this progress. Some of these limitations are connected to the fact, that the ablation process of a~sample is fast and dynamic and the changes of the plasma plume in time and space are a question of a few microseconds. As this can cause certain limitations in the analysis process, there has been a question of how to minimize or eliminate these problems. For this purpose, supplementary methods have been more and more implemented in the LIBS experiments. The goal is simple, acquire more information from the complex process of the ablation and improve the analytical performance of LIBS, be it in the scope of qualitative or quantitative analysis. Here lies the main motivation of this dissertation thesis. Goal of this thesis was to research, implement and utilize supplementary methods, that could be used in combination with the existing LIBS experimental setup. As a result, direct plasma imaging, shadowgraphy and sound analysis systems have been implemented and streamlined into the typical analytical process. Each of these methods brings certain additional information. For direct plasma imaging, it can be the spacious-temporal morphology of the plasma plume, or the distribution of individual elements within its volume. The Shadowgraphy method can be used to calculate the energy spent on the ablation itself, pointing at the thermal properties of the analyzed sample. Lastly, the sound information from the generated shock wave is connected to the amount of ablated mass. Within this thesis, all of the mentioned supplementary methods were examined, and utilized. Insight into these methods together with the LIBS analysis was done individually for each method as well as from the point of their mutual combination. The theoretical information as well as their background is described and discussed. Moreover, the technical information is discussed and analyzed, be it the implementation of the LIBS experiment, or the actual data analysis process. This work will serve as a foundation for further research in this area, where a selection of these methods will be used in several applications that are already using LIBS but suffer from certain limitations. These methods will be used to mitigate the limitation and to elevate the potential use of the LIBS in certain areas and applications.en
dc.description.abstractLaser-Induced Breakdown Spectroscopy (LIBS) is a method of analytical chemistry that provides a qualitative and quantitative sample analysis. As this method has been implemented in more and more applications, certain limitations and drawbacks have been raised from this progress. Some of these limitations are connected to the fact, that the ablation process of a~sample is fast and dynamic and the changes of the plasma plume in time and space are a question of a few microseconds. As this can cause certain limitations in the analysis process, there has been a question of how to minimize or eliminate these problems. For this purpose, supplementary methods have been more and more implemented in the LIBS experiments. The goal is simple, acquire more information from the complex process of the ablation and improve the analytical performance of LIBS, be it in the scope of qualitative or quantitative analysis. Here lies the main motivation of this dissertation thesis. Goal of this thesis was to research, implement and utilize supplementary methods, that could be used in combination with the existing LIBS experimental setup. As a result, direct plasma imaging, shadowgraphy and sound analysis systems have been implemented and streamlined into the typical analytical process. Each of these methods brings certain additional information. For direct plasma imaging, it can be the spacious-temporal morphology of the plasma plume, or the distribution of individual elements within its volume. The Shadowgraphy method can be used to calculate the energy spent on the ablation itself, pointing at the thermal properties of the analyzed sample. Lastly, the sound information from the generated shock wave is connected to the amount of ablated mass. Within this thesis, all of the mentioned supplementary methods were examined, and utilized. Insight into these methods together with the LIBS analysis was done individually for each method as well as from the point of their mutual combination. The theoretical information as well as their background is described and discussed. Moreover, the technical information is discussed and analyzed, be it the implementation of the LIBS experiment, or the actual data analysis process. This work will serve as a foundation for further research in this area, where a selection of these methods will be used in several applications that are already using LIBS but suffer from certain limitations. These methods will be used to mitigate the limitation and to elevate the potential use of the LIBS in certain areas and applications.cs
dc.description.markPcs
dc.identifier.citationBUDAY, J. Studie evoluce laserem indukovaného plazmatu pomocí komplementárních a spektroskopických metod [online]. Brno: Vysoké učení technické v Brně. Fakulta strojního inženýrství. .cs
dc.identifier.other154820cs
dc.identifier.urihttps://hdl.handle.net/11012/249183
dc.language.isoencs
dc.publisherVysoké učení technické v Brně. Fakulta strojního inženýrstvícs
dc.rightsStandardní licenční smlouva - přístup k plnému textu bez omezenícs
dc.subjectLaser-Induced Breakdown Spectroscopyen
dc.subjectLIBSen
dc.subjectLaser-Induced Plasmaen
dc.subjectLIPen
dc.subjectspectroscopyen
dc.subjectplasma imagingen
dc.subjectShadowgraphyen
dc.subjectsound analysisen
dc.subjectsupplementary method analysisen
dc.subjectdata statisticsen
dc.subjectdata correlationen
dc.subjectLaser-Induced Breakdown Spectroscopycs
dc.subjectLIBScs
dc.subjectLaser-Induced Plasmacs
dc.subjectLIPcs
dc.subjectspectroscopycs
dc.subjectplasma imagingcs
dc.subjectShadowgraphycs
dc.subjectsound analysiscs
dc.subjectsupplementary method analysiscs
dc.subjectdata statisticscs
dc.subjectdata correlationcs
dc.titleStudie evoluce laserem indukovaného plazmatu pomocí komplementárních a spektroskopických metoden
dc.title.alternativeInvestigating the evolution of laser induced plasmas by complementary optical and spectroscopic methodscs
dc.typeTextcs
dc.type.driverdoctoralThesisen
dc.type.evskpdizertační prácecs
dcterms.modified2024-07-03-13:43:13cs
eprints.affiliatedInstitution.facultyFakulta strojního inženýrstvícs
sync.item.dbid154820en
sync.item.dbtypeZPen
sync.item.insts2024.07.04 05:58:30en
sync.item.modts2024.07.04 05:12:41en
thesis.disciplineFyzikální a materiálové inženýrstvícs
thesis.grantorVysoké učení technické v Brně. Fakulta strojního inženýrství. Ústav fyzikálního inženýrstvícs
thesis.levelDoktorskýcs
thesis.namePh.D.cs
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