Destructive Photon Echo Formation in Six-Wave Mixing Signals of a MoSe2 Monolayer

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dc.contributor.authorHahn, Thilocs
dc.contributor.authorVáclavková, Dianacs
dc.contributor.authorBartoš, Miroslavcs
dc.contributor.authorNogajewski, Karolcs
dc.contributor.authorPotemski, Marekcs
dc.contributor.authorWatanabe, Kenjics
dc.contributor.authorTaniguchi, Takashics
dc.contributor.authorMachnikowski, Pawełcs
dc.contributor.authorKuhn, Tilmanncs
dc.contributor.authorKasprzak, Jacekcs
dc.contributor.authorWigger, Danielcs
dc.coverage.issue1cs
dc.coverage.volume9cs
dc.date.accessioned2022-01-11T11:54:34Z
dc.date.available2022-01-11T11:54:34Z
dc.date.issued2022-01-05cs
dc.description.abstractMonolayers of transition metal dichalcogenides display a strong excitonic optical response. Additionally encapsulating the monolayer with hexagonal boron nitride allows to reach the limit of a purely homogeneously broadened exciton system. On such a MoSe2-based system, ultrafast six-wave mixing spectroscopy is performed and a novel destructive photon echo effect is found. This process manifests as a characteristic depression of the nonlinear signal dynamics when scanning the delay between the applied laser pulses. By theoretically describing the process within a local field model, an excellent agreement with the experiment is reached. An effective Bloch vector representation is developed and thereby it is demonstrated that the destructive photon echo stems from a destructive interference of successive repetitions of the heterodyning experiment.en
dc.formattextcs
dc.format.extent1-13cs
dc.format.mimetypeapplication/pdfcs
dc.identifier.citationAdvanced Science. 2022, vol. 9, issue 1, p. 1-13.en
dc.identifier.doi10.1002/advs.202103813cs
dc.identifier.issn2198-3844cs
dc.identifier.other174114cs
dc.identifier.urihttp://hdl.handle.net/11012/203282
dc.language.isoencs
dc.publisherWiley-VCHcs
dc.relation.ispartofAdvanced Sciencecs
dc.relation.urihttps://onlinelibrary.wiley.com/doi/10.1002/advs.202103813cs
dc.rightsCreative Commons Attribution 4.0 Internationalcs
dc.rights.accessopenAccesscs
dc.rights.sherpahttp://www.sherpa.ac.uk/romeo/issn/2198-3844/cs
dc.rights.urihttp://creativecommons.org/licenses/by/4.0/cs
dc.subjectnonlinear spectroscopyen
dc.subjectphoton echoen
dc.subjecttransition metal dichalcogenidesen
dc.titleDestructive Photon Echo Formation in Six-Wave Mixing Signals of a MoSe2 Monolayeren
dc.type.driverarticleen
dc.type.statusPeer-revieweden
dc.type.versionpublishedVersionen
sync.item.dbidVAV-174114en
sync.item.dbtypeVAVen
sync.item.insts2022.06.15 12:52:18en
sync.item.modts2022.06.15 12:14:18en
thesis.grantorVysoké učení technické v Brně. Středoevropský technologický institut VUT. Magneto-Optická a THz Spektroskopiecs
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